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澶嶅悎鏉愭枡
褰撳墠浣嶇疆錛?棣栭〉 >> 璧勮 >> 澶嶅悎鏉愭枡 >> 琛屼笟鍔ㄦ?/a> >> 姝ｆ枃

浣?/span>涓?/span>褰?/span>浠?/span>鏈鍙?/span>鑰?/span>鐨?/span>縐?/span>瀛?/span>闂?/span>棰?/span>涔?/span>涓鐨?/span>鎺?/span>瑙?/span>璧?/span>鐢?/span>錛?/span>鏈鏃?/span>鏄?/span>鍦?/span>綰?/span>2600騫?/span>鍓?/span>鐨?/span>鍙?/span>甯?/span>鑵?/span>鍙?/span>鐜?/span>錛?/span>铏?/span>鐒?/span>榪?/span>鏄?/span>浜?/span>浠?/span>姣?/span>澶?/span>涓?/span>鍙?/span>閬?/span>鍏?/span>閮?/span>浼?/span>緇?/span>鍘?/span>鐨?/span>鐜?/span>璞?/span>錛?/span>浣?/span>瀹?/span>鑳?/span>鍚?/span>鐨?/span>鐗?/span>鐞?/span>鏈?/span>鍒?/span>渚?/span>鐒?/span>鎮?/span>鑰?/span>鏈?/span>鍐?/span>錛?/span>涓鐩?/span>瀛?/span>鍦?/span>浜?/span>璁?/span>銆?/span>鑰?/span>鍩?/span>浜?/span>鎺?/span>瑙?/span>璧?/span>鐢?/span>鍜?/span>闈?/span>鐢?/span>璇?/span>瀵?/span>鏁?/span>搴?/span>鑰?/span>鍙?/span>鏄?/span>鐨?/span>鎽?/span>鎿?/span>綰?/span>綾?/span>鍙?/span>鐢?/span>鏈?/span>錛?/span>TENG錛?/span>浣?/span>涓?/span>涓欏?/span>鏂?/span>鍏?/span>鐨?/span>鎶鏈?/span>錛?/span>涓?/span>浜?/span>浠?/span>瑙?/span>鍐?/span>涓?/span>鐣?/span>鑳?/span>婧?/span>闂?/span>棰?/span>鎻?/span>渚?/span>浜?/span>涓涓?/span>鏂?/span>鐨?/span>閫?/span>欏?/span>錛?/span>鎺?/span>瑙?/span>璧?/span>鐢?/span>涔?/span>鎴?/span>涓?/span>褰?/span>鍓?/span>鐨?/span>鐮?/span>絀?/span>鐑?/span>鐐?/span>涔?/span>涓銆?/span>


涓?/span>鍥?/span>鐭?/span>涓?/span>澶?/span>瀛?/span>璁?/span>紼?/span>鍓?/span>鏁?/span>鎺?/span>鍜?/span>涓?/span>縐?/span>闄?/span>鍖?/span>浜?/span>綰?/span>綾?/span>鑳?/span>婧?/span>涓?/span>緋?/span>緇?/span>鐮?/span>絀?/span>鎵鐜?/span>涓?/span>鏋?/span>闄?/span>澹?/span>鍦?/span>銆?/span>ACS Applied Materials & Interfaces銆?/span>鏈?/span>鍒?/span>涓?/span>鍙?/span>琛?/span>浜?/span>棰?/span>涓?/span>鈥?/span>Effects of Oxygen Vacancies and Cation Valence States on the Triboelectric Property of Substoichiometric Oxide Films鈥?/span>鐨?/span>鏂?/span>绔?/span>錛?/span>DOI: 10.1021/acsami.1c09248錛?/span>銆?/span>涓?/span>浜?/span>鎺?/span>绱?/span>娓?/span>搴?/span>瀵?/span>浜?/span>鎺?/span>瑙?/span>璧?/span>鐢?/span>鐨?/span>褰?/span>鍝?/span>錛?/span>璇?/span>璇?/span>棰?/span>緇?/span>閲?/span>鐢?/span>鐢?/span>瀛?/span>鏉?/span>钂?/span>鍙?/span>鏂?/span>娉?/span>鍒?/span>澶?/span>浜?/span>涓?/span>鍚?/span>縐?/span>綾?/span>鐨?/span>浜?/span>鍖?/span>瀛?/span>璁?/span>閲?/span>姣?/span>姘?/span>鍖?/span>鐗?/span>钖?/span>鑶?/span>錛?/span>騫?/span>榪?/span>琛?/span>浜?/span>涓?/span>鍚?/span>娓?/span>搴?/span>鐨?/span>閫鐏?/span>鍚?/span>澶?/span>鐞?/span>銆?/span>闅?/span>鐫鍦?/span>絀?/span>姘?/span>涓?/span>閫鐏?/span>娓?/span>搴?/span>鐨?/span>鎻?/span>楂?/span>錛?/span>寮灝?/span>鏂?/span>鎺?/span>閽?/span>鍔?/span>鏄?/span>寰?/span>闀?/span>嫻?/span>璇?/span>緇?/span>鏋?/span>琛?/span>鏄?/span>TiO2-x鐨?/span>寰?/span>鍖?/span>鎺?/span>瑙?/span>璧?/span>鐢?/span>鐗?/span>鎬?/span>鍙?/span>鐢?/span>浜?/span>鐢?/span>璐?/span>鐢?/span>鑽?/span>鍚?/span>姝?/span>鐢?/span>鑽?/span>鏂?/span>鍚?/span>杞?/span>鍙?/span>鐨?/span>鏈?/span>瓚?/span>鐜?/span>璞?/span>銆?/span>鍥?/span>涓?/span>絀?/span>姘?/span>灞?/span>浜?/span>姘?/span>鍖?/span>鎬?/span>姘?/span>姘?/span>錛?/span>璇?/span>鏉?/span>浠?/span>涓?/span>閫鐏?/span>淇?/span>澶?/span>浜?/span>姘?/span>絀?/span>浣?/span>騫?/span>涓?/span>鏈?/span>鍒?/span>浜?/span>鎻?/span>鍗?/span>浣?/span>鍖?/span>瀛?/span>浠?/span>鐨?/span>Ti3 鑷?/span>紼?/span>瀹?/span>鐨?/span>楂?/span>浠?/span>Ti4 銆?/span>涓?/span>涔?/span>鐩?/span>鍙?/span>錛?/span>濡?/span>鏋?/span>鍦?/span>Ar/H2姘?/span>姘?/span>涓?/span>閫鐏?/span>錛?/span>鍒?/span>浼?/span>浣?/span>寰?/span>钖?/span>鑶?/span>鐨?/span>璧?/span>鐢?/span>鐢?/span>姝?/span>鐢?/span>鑽?/span>鍚?/span>璐?/span>鐢?/span>鑽?/span>鏂?/span>鍚?/span>鍙?/span>鍖?/span>銆?/span>榪?/span>鏄?/span>鐢?/span>浜?/span>鍦?/span>榪?/span>鍘?/span>鎬?/span>姘?/span>姘?/span>鏉?/span>浠?/span>涓?/span>閫鐏?/span>錛?/span>浣?/span>寰?/span>姘?/span>絀?/span>浣?/span>澧?/span>鍔?/span>浜?/span>銆?/span>閫?/span>榪?/span>瀵?/span>Al2O3-x, Ta2O5-x鍜?/span>Cr2O3-x絳?/span>浜?/span>鍖?/span>瀛?/span>璁?/span>閲?/span>姣?/span>姘?/span>鍖?/span>鐗?/span>钖?/span>鑶?/span>鐨?/span>鐮?/span>絀?/span>錛?/span>榪?/span>涓姝?/span>楠?/span>璇?/span>浜?/span>姘?/span>絀?/span>浣?/span>鐨?/span>浣?/span>鐢?/span>錛?/span>鍗?/span>姘?/span>絀?/span>浣?/span>鍑?/span>灝?/span>灝?/span>淇?/span>浣?/span>钖?/span>鑶?/span>鐨?/span>琛?/span>闈?/span>璧?/span>鐢?/span>鐗?/span>鎬?/span>浠?/span>鐢?/span>璐?/span>鐢?/span>鑽?/span>鍚?/span>姝?/span>鐢?/span>鑽?/span>鏂?/span>鍚?/span>杞?/span>鍙?/span>銆?/span>閲?/span>鐢?/span>姝?/span>鍒?/span>鐢?/span>綆鍗?/span>鐨?/span>閫鐏?/span>澶?/span>鐞?/span>鏂?/span>寮?/span>錛?/span>鐮?/span>鍒?/span>鍑?/span>浜?/span>鑳?/span>澶?/span>鎺?/span>鍒?/span>鐢?/span>嫻?/span>鏂?/span>鍚?/span>鐨?/span>鍚?/span>縐?/span>鏉?/span>鏂?/span>IM鈥?/span>TENGs銆?/span>鏈鍚?/span>錛?/span>鍩?/span>浜?/span>瀹?/span>楠?/span>緇?/span>鏋?/span>錛?/span>鎻?/span>鍑?/span>浜?/span>閲?/span>灞?/span>涓?/span>涓?/span>鍚?/span>娓?/span>搴?/span>閫鐏?/span>鍚?/span>鐨?/span>鐢?/span>浠?/span>璐?/span>鐨?/span>鎺?/span>瑙?/span>璧?/span>鐢?/span>鐨?/span>琛?/span>闈?/span>鎬?/span>妯?/span>鍨?/span>錛?/span>鎻?/span>紺?/span>浜?/span>姘?/span>絀?/span>浣?/span>涓?/span>瑕?/span>鏄?/span>閫?/span>榪?/span>瀵?/span>琛?/span>闈?/span>鎬?/span>涓?/span>鏉?/span>緙?/span>鐢?/span>瀛?/span>鑳?/span>閲?/span>鐨?/span>褰?/span>鍝?/span>錛?/span>浠?/span>鑰?/span>鍐?/span>瀹?/span>浜?/span>鍚?/span>緇?/span>鐨?/span>鐢?/span>瀛?/span>杞?/span>縐?/span>騫?/span>浜?/span>鐢?/span>鎺?/span>瑙?/span>璧?/span>鐢?/span>銆?/span>璇?/span>鐮?/span>絀?/span>鏈?/span>鍒?/span>浜?/span>鏈?/span>鏉?/span>寮鍙?/span>鍑?/span>鑳?/span>澶?/span>綺?/span>紜?/span>鎺?/span>鍒?/span>鐢?/span>嫻?/span>鏂?/span>鍚?/span>鎴?/span>鐢?/span>鍘?/span>澶?/span>灝?/span>鐨?/span>鍚?/span>鏉?/span>璐?/span>IM鈥?/span>TENGs錛?/span>鍚?/span>鏃?/span>涔?/span>涓?/span>鎺?/span>瑙?/span>璧?/span>鐢?/span>涓?/span>鐨?/span>鐢?/span>瀛?/span>杞?/span>縐?/span>涓?/span>瀵?/span>鏈?/span>鍒?/span>鎻?/span>渚?/span>浜?/span>鏇?/span>榪?/span>涓姝?/span>鐨?/span>鐞?/span>瑙?/span>銆?/span>


鍥?/span>1 閲?/span>鐢?/span>20 sccm姘?/span>姘?/span>娌?/span>縐?/span>鐨?/span>TiO2-x钖?/span>鑶?/span>鐨?/span>鎬?/span>鑳?/span>鍙?/span>鍖?/span>鍙?/span>鎽?/span>鎿?/span>鐢?/span>鑽?/span>婕?/span>鍖?/span> (a) 钖?/span>鑶?/span>琛?/span>闈?/span>褰?/span>璨?/span> (b) XRD緇?/span>鏋?/span> (c) 钖?/span>鑶?/span>鍘?/span>搴?/span> (d-e) 钖?/span>鑶?/span>琛?/span>闈?/span>Ti2p鍜?/span>O1s鐨?/span>XPS璋?/span> (f) 瀹?/span>娓?/span>涓?/span>鍦?/span>絀?/span>姘?/span>涓?/span>閫鐏?/span>鍓?/span>鍚?/span>钖?/span>鑶?/span>鐨?/span>鎽?/span>鎿?/span>鐢?/span>鑽?/span>瀵?/span>搴?/span>銆?/span>



鍥?/span>2 閲?/span>鐢?/span>80 sccm姘?/span>姘?/span>娌?/span>縐?/span>鐨?/span>TiO2-x钖?/span>鑶?/span>鎽?/span>鎿?/span>鐢?/span>鑽?/span>婕?/span>鍖?/span> (a)絀?/span>姘?/span>涓?/span>涓?/span>鍚?/span>娓?/span>搴?/span>閫鐏?/span>鍓?/span>鍚?/span>钖?/span>鑶?/span>鍦?/span>瀹?/span>娓?/span>涓?/span>鐨?/span>鎽?/span>鎿?/span>鐢?/span>鑽?/span>瀵?/span>搴?/span> (b) 钖?/span>鑶?/span>琛?/span>闈?/span>Ti2p鐨?/span>XPS璋?/span> (c) 钖?/span>鑶?/span>鍘?/span>搴?/span> (d) 涓?/span>鍚?/span>閫鐏?/span>鏉?/span>浠?/span>涓?/span>澶?/span>鐞?/span>鍚?/span>鐨?/span>钖?/span>鑶?/span>鍦?/span>瀹?/span>娓?/span>涓?/span>鐨?/span>鎽?/span>鎿?/span>鐢?/span>鑽?/span>瀵?/span>搴?/span>銆?/span>


鍥?/span>3 Al2O3-x钖?/span>鑶?/span>鐨?/span>鎬?/span>鑳?/span>鍙?/span>鍖?/span>涓?/span>鎽?/span>鎿?/span>鐢?/span>鑽?/span>婕?/span>鍖?/span> (a) 钖?/span>鑶?/span>琛?/span>闈?/span>褰?/span>璨?/span> (b) XRD緇?/span>鏋?/span> (c) 钖?/span>鑶?/span>琛?/span>闈?/span> (c-d) Al2p鍜?/span>O1s鐨?/span>XPS璋?/span> (e) 瀹?/span>娓?/span>涓?/span>5 sccm姘?/span>姘?/span>娌?/span>縐?/span>钖?/span>鑶?/span>鐨?/span>鎽?/span>鎿?/span>鐢?/span>鑽?/span>瀵?/span>搴?/span> (f) 瀹?/span>娓?/span>涓?/span>20 sccm姘?/span>姘?/span>娌?/span>縐?/span>钖?/span>鑶?/span>鐨?/span>鎽?/span>鎿?/span>鐢?/span>鑽?/span>瀵?/span>搴?/span>銆?/span>


鍥?/span>4 Ta2O5-x鍜?/span>Cr2O3-x钖?/span>鑶?/span>鐨?/span>鎬?/span>鑳?/span>鍙?/span>鍖?/span>鍜?/span>鎽?/span>鎿?/span>鐢?/span>鑽?/span>婕?/span>鍖?/span> (a) 閫鐏?/span>鍓?/span>鍚?/span>Ta2O5-x钖?/span>鑶?/span>鐨?/span>XRD緇?/span>鏋?/span> (b) 閫鐏?/span>鍓?/span>鍚?/span>Ta2O5-x钖?/span>鑶?/span>琛?/span>闈?/span>Ta4f鐨?/span>XPS璋?/span> (c) 瀹?/span>娓?/span>涓?/span>Ta2O5-x钖?/span>鑶?/span>鐨?/span>鎽?/span>鎿?/span>鐢?/span>鑽?/span>瀵?/span>搴?/span> (d) Cr2O3-x钖?/span>鑶?/span>閫鐏?/span>鍓?/span>鍚?/span>鐨?/span>XRD緇?/span>鏋?/span> (e) Cr2O3-x钖?/span>鑶?/span>琛?/span>闈?/span>鐨?/span>Cr2p鐨?/span>XPS璋?/span> (f) 瀹?/span>娓?/span>涓?/span>Cr2O3-x钖?/span>鑶?/span>鐨?/span>鎽?/span>鎿?/span>鐢?/span>鑽?/span>瀵?/span>搴?/span>銆?/span>


鍥?/span>5 TiO2-x鍩?/span>鍚?/span>鏉?/span>璐?/span>IM-TENGs鐨?/span>鎬?/span>鑳?/span> (a) IM-TENGs鐨?/span>紺?/span>鎰?/span>鍥?/span> (b-c) 鐢?/span>閫鐏?/span>鍓?/span>鍜?/span>573 K閫鐏?/span>鍚?/span>鐨?/span>TiO2-x钖?/span>鑶?/span>鍒?/span>鎴?/span>鐨?/span>IM-TENG鐨?/span>VOC鍜?/span>QSC (d-e) 鐢?/span>573 K閫鐏?/span>鍚?/span>鐨?/span>TiO2-x钖?/span>鑶?/span>鍒?/span>鎴?/span>鐨?/span>IM-TENG鐨?/span>VOC鍜?/span>QSC (f) 涓?/span>鍚?/span>緇?/span>鐨?/span>IM-TENGs鐨?/span>VOC銆?/span>


鍥?/span>6 鐢?/span>浜?/span>瑙?/span>閲?/span>閲?/span>灞?/span>鍜?/span>鐢?/span>浠?/span>璐?/span>鍦?/span>涓?/span>鍚?/span>娓?/span>搴?/span>涓?/span>閫鐏?/span>鐨?/span>鎺?/span>瑙?/span>璧?/span>鐢?/span>鏈?/span>鍒?/span>鐨?/span>琛?/span>闈?/span>鎬?/span>妯?/span>鍨?/span> (a-c) 閲?/span>灞?/span>鍜?/span>閫鐏?/span>鍓?/span>鐢?/span>浠?/span>璐?/span>涔?/span>闂?/span>鐨?/span>鐢?/span>鑽?/span>杞?/span>縐?/span> (d-f) 閲?/span>灞?/span>鍜?/span>T1娓?/span>搴?/span>閫鐏?/span>鍚?/span>鐢?/span>浠?/span>璐?/span>涔?/span>闂?/span>鐨?/span>鐢?/span>鑽?/span>杞?/span>縐?/span> (g-i) 閲?/span>灞?/span>鍜?/span>T2娓?/span>搴?/span>閫鐏?/span>鍚?/span>鐢?/span>浠?/span>璐?/span>涔?/span>闂?/span>鐨?/span>鐢?/span>鑽?/span>杞?/span>縐?/span>銆?/span>T1<T2銆?/span>


鐩?/strong>鍏?/strong>閾?/strong>鎺?/strong>

https://pubs.acs.org/doi/full/10.1021/acsami.1c09248

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